Like they said. The square one is the charcoal canister to capture gas fumes from the tank vent.
Its smog related. If you are ever likely to have to pass smog, don't take it off.
The round one is usually important. Its nothing but a hollow ball, but if you have vacuum controlled anything, its needed to supply vacuum when the engine is not making much.
Had a '71 T-bird. Vacuum everything.
It had two coffee can sized vacuum reservoirs.
One of them developed a leak.
In the middle of summer, 90 degrees in the shade, the climate control system would go from full cool to full heat when you stepped on the gas........